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Controlling the Abruptness of Axial Heterojunctions in III-V Nanowires: Beyond the Reservoir Effect

Författare

Summary, in English

Heterostructure nanowires have many potential applications due to the avoidance of interface defects by lateral strain relaxation. However, most heterostructure semiconductor nanowires suffer from persistent interface compositional grading, normally attributed to the dissolution of growth species in the common alloy seed particles. Although progress has been made for some material systems, most binary material combinations remain problematic due to the interaction of growth species in the alloy. In this work we investigate the formation of interfaces in InAs-GaAs heterostructures experimentally and theoretically and demonstrate a technique to attain substantially sharper interfaces. We show that by pulsing the Ga source during heterojunction formation, In is pushed out before GaAs growth initiates, greatly reducing In carry-over. This procedure will be directly applicable to any nanowire system with finite nonideal solubility of growth species in the alloy seed particle and greatly improve the applicability of these structures in future devices.

Publiceringsår

2012

Språk

Engelska

Sidor

3200-3206

Publikation/Tidskrift/Serie

Nano Letters

Volym

12

Issue

6

Dokumenttyp

Artikel i tidskrift

Förlag

The American Chemical Society (ACS)

Ämne

  • Nano Technology

Nyckelord

  • Nanowire
  • heterostructure
  • III-V semiconductor
  • MOVPE
  • XEDS

Status

Published

ISBN/ISSN/Övrigt

  • ISSN: 1530-6992