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Development of multipoint vibrational coherent anti-Stokes Raman spectroscopy for flame applications

In English

Författare

Summary, in English

A novel technique for coherent anti-Stokes Raman spectroscopy (CARS) measurements in multiple points is presented. In a multipass cavity the pump and Stokes laser beams are multiply reflected and refocused into a measurement volume with an adjustable number of separated points along a line. This optical arrangement was used in a vibrational CARS setup with planar BOXCARS phase-matching configuration. The CARS spectra from spatially separated points were recorded at different heights on a CCD camera. Measurements of temperature profiles were carried out in the burned gas zone of a premixed one-dimensional flame to demonstrate the applicability of this method for temperature measurements in high-temperature regions. The ability to measure in flames with strong density gradients was demonstrated by simultaneous measurements of Q-branch spectra of N-2 and CO in a Wolfhard-Parker burner flame. Interference phenomena found in multipoint spectra are discussed, and possible solutions are proposed. Merits and limitations of the technique are discussed. (c) 2006 Optical Society of America.

Publiceringsår

2006

Språk

Engelska

Sidor

1177-1186

Publikation/Tidskrift/Serie

Applied Optics

Volym

45

Issue

6

Dokumenttyp

Artikel i tidskrift

Förlag

Optical Society of America

Ämne

  • Atom and Molecular Physics and Optics

Status

Published

ISBN/ISSN/Övrigt

  • ISSN: 2155-3165